The technique of scanning tunneling microscopy (STM) with a normal metal tip has recently been used to study the high transition temperature ( TC) superconducting cuprates and has revealed many fascinating and complex features of quasiparticle excited states of these materials. For conventional superconductors, the Bardeen-Cooper-Schrieffer theory connects the pair amplitude and the superconducting gap as measured from the quasiparticle excitation spectra, while for the high-TC materials there is still no theory to connect these quantities. We are unable to make any quantitative analysis of the superconducting ground state from the quasiparticle data.
Josephson tunneling is the tunneling of the Cooper pairs between two superconductors and the Josephson current directly relates to the superconducting pair wave function amplitude. In this thesis, we have developed the superconducting STM as a local Josephson probe and carried out direct measurements of the superconducting pair amplitude of Bi2Sr2CaCu2O 8+δ single crystals via the c-axis Josephson tunneling between Bi2Sr2CaCu2O8+δ and a conventional superconducting STM tip. Josephson measurements at different surface locations of overdoped Bi2Sr2CaCu 2O8+δ yield local values for the Josephson ICRN product, indicating an inhomogeneous structure of the ICRN product in overdoped Bi 2Sr2CaCu2O8+δ on a nanometer length scale. The corresponding energy gap, Δ, was also measured at the same locations and an unexpected inverse correlation is observed between the local ICRN product and the local energy gap Δ. Our interpretation of the ICR N vs. Δ relation with the phase fluctuation model for the phase diagram of high-TC superconducting cuprates will be presented.
A preliminary study of the high current density effect on the density of states of Bi2Sr2CaCu2O8+δ will also be reported.
The effect of cleaving the Bi2Sr2CaCu2O 8+δ surface on its electronic structure is also discussed. This is motivated by the question that the gap inhomogeneity observed by STM is intrinsic property of this material or induced by the cleaving. Since the superconducting tunneling probes the depth of a coherence length into the sample surface and Bi2Sr2CaCu2O 8+δ has a very short c-axis coherence length, it’s important to address this question. I will present some preliminary results of the superconducting STM studies on chemically etched Bi2Sr 2CaCu2O8+δ surfaces.
|Advisor:||Dynes, Robert C.|
|Commitee:||Crommie, Michael F., Suzuki, Yuri|
|School:||University of California, Berkeley|
|School Location:||United States -- California|
|Source:||DAI-B 71/12, Dissertation Abstracts International|
|Subjects:||Inorganic chemistry, Condensed matter physics, Materials science|
|Keywords:||High-tc superconducting cuprates, Josephson effect, Superconducting order, Superconductors|
Copyright in each Dissertation and Thesis is retained by the author. All Rights Reserved
The supplemental file or files you are about to download were provided to ProQuest by the author as part of a
dissertation or thesis. The supplemental files are provided "AS IS" without warranty. ProQuest is not responsible for the
content, format or impact on the supplemental file(s) on our system. in some cases, the file type may be unknown or
may be a .exe file. We recommend caution as you open such files.
Copyright of the original materials contained in the supplemental file is retained by the author and your access to the
supplemental files is subject to the ProQuest Terms and Conditions of use.
Depending on the size of the file(s) you are downloading, the system may take some time to download them. Please be